Quantum phases of cold polar molecules in 2D optical lattices

We study the quantum phases of hard-core bosonic polar molecules on a two-dimensional square lattice interacting via repulsive dipole-dipole interactions. In the limit of small tunneling, we find evidence for a devil's staircase, where Mott solids appear at rational fillings of the lattice. For finite tunneling, we establish the existence of extended regions of parameters where the ground state is a supersolid, obtained by doping the solids either with particles or vacancies. We discuss the effects of finite temperature and finite-size confining potentials as relevant to experiments. © 2010 The American Physical Society.